Sounds ok. Just be ready for a bit of potential shock to the system when you start Sustained Power Build. That’s lots of Threshold work on the heels of much lower intensity work. You’ll have a decent base, but the RPE may be a jump.
LR100 for nearly all of us is about survival. Therefore you want to be able to put out watts consistently for as long as possible. I would say mid volume sweet spot with as long as possible rides on the weekend. The ability to ride at 70% - 80% of FTP for 5hrs will put you in the front half of the ride. Personally I would focus on sweet spot over anything for someone looking to complete.
Also gym work to prepare for those likely hike a bike sections.
Last year I started with SSB mid and moved to Sustained Power Build mid rolling into the race. If it’s a mud year like 2017, be prepared for anything and everything you could imagine being thrown at you…it adds to the adventure though.
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